TIAN Qing,JI Yan-qin,YIN Liang-liang,HUANG Wei,SHAO Xian-zhang,SHEN Bao-ming.Determination by ICP-MS of uranium isotopic ratios in drinking water in the vicinity of nuclear power plants[J].Chinese Journal of Radiological Medicine and Protection,2013,33(1):72-75
Determination by ICP-MS of uranium isotopic ratios in drinking water in the vicinity of nuclear power plants
Received:April 09, 2012  
DOI:10.3760/cma.j.issn.0254-5098.2013.01.020
KeyWords:Uranium  Inductively coupled plasma mass spectrometry  Isotope ratios  Surface water
FundProject:卫生行业科研专项(201002009)
Author NameAffiliationE-mail
TIAN Qing Key Laboratory of Radiological Protection and Nuclear Emergency, China CDC, National Institute for Radiological Protection, Chinese Center for Disease Control and Prevention, Beijing 100088, China  
JI Yan-qin Key Laboratory of Radiological Protection and Nuclear Emergency, China CDC, National Institute for Radiological Protection, Chinese Center for Disease Control and Prevention, Beijing 100088, China jiyanqin@nirp.cn 
YIN Liang-liang Key Laboratory of Radiological Protection and Nuclear Emergency, China CDC, National Institute for Radiological Protection, Chinese Center for Disease Control and Prevention, Beijing 100088, China  
HUANG Wei Key Laboratory of Radiological Protection and Nuclear Emergency, China CDC, National Institute for Radiological Protection, Chinese Center for Disease Control and Prevention, Beijing 100088, China  
SHAO Xian-zhang Key Laboratory of Radiological Protection and Nuclear Emergency, China CDC, National Institute for Radiological Protection, Chinese Center for Disease Control and Prevention, Beijing 100088, China  
SHEN Bao-ming Key Laboratory of Radiological Protection and Nuclear Emergency, China CDC, National Institute for Radiological Protection, Chinese Center for Disease Control and Prevention, Beijing 100088, China  
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Abstract::
      Objective To ascertain the uranium isotopic ratios in surface water samples around nuclear power plants. Methods Water samples were collected in Jiangsu, Shandong and Zhejiang provinces. An efficient separation procedure for the trace uranium concentrated from surface water by tributyl phosphate (TBP) was used. Inductively coupled plasma mass spectrometry (ICP-MS) was applied to determination of low abundance uranium isotopes. Results The 234U/238U isotope ratio varied from 4.575×10-5 to 7.752×10-5 and 235U/238U from 7.273×10-3 to 7.639×10-3. Conclusions The 234U is enriched in the surface water.
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